If you saw a cover letter in iambic pentameter, would that turn you off?
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I'd appreciate it... but I probably wouldn't send that to anyone. I've left some "arty" YouTube comments in the past and at least half the time people don't even understand what you're doing.
I have an app on my phone whose update notes are always in haiku. :D
On review, I found what I'd written (footed; not metered) was a synopsis.